Slow-Neutron Scattering by Water

TL;DRAbstract

Experimental data on the slow-neutron ( < 0.1 eV) scattering of room-temperature water have been obtained using the velocity selector at the Materials Testing Reactor. The data agree with the results of Haywood obtained using a slow-neutron velocity selector, with the results of Kottwitz and Leonard obtained using a triple-axis spectrometer, and with the results of Kirouac obtained using a linear accelerator plus phased chopper. There are marked differences from the results of Sakamoto and co-workers, who used cold neutrons and a rotating crystal spectrometer. An extension of the Nelkin model has been devised that gives calculated results in good agreement with the MTR data, whereas the Nelkin model generally gives poor agreement. The new model treats water as a mixture of 10% of free molecules and 45% each of two aggregates in which the effective masses for H scattering are 75 and 150. Each aggregate has a set of vibrational modes with energies distributed in the range 0 < E ≤ 0.125 e

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